@article{6322,
  author = {S. Roke and A. W. Kleyn and M. Bonn},
  title = {Time- vs. frequency-domain femtosecond surface sum frequency generation},
  abstract = {We present an experimental and theoretical investigation into time- vs. frequency-domain ferntosecond sum frequency spectroscopy at the metal-liquid interface. Although frequency and time-domain measurements are theoretically equivalent it is demonstrated here experimentally that the two approaches are sensitive to different physical aspects of the system and provide complementary information. Time-domain measurements are demonstrated to be more clearly influenced by the inhomogeneity of adsorption sites, since the decay of the vibrational polarization can be mapped directly. A generalization of existing models allows for the simultaneous description of both frequency and time-domain measurements. (C) 2003 Elsevier Science B.V. All rights reserved.},
  year = {2003},
  journal = {Chemical Physics Letters},
  volume = {370},
  number = {1-2},
  pages = {227-232},
  note = {Using Smart Source Parsing7},
  language = {eng},
}