Plasma assisted nitrogen oxide production from air: Using pulsed powered gliding arc reactor for a containerized plant

TitlePlasma assisted nitrogen oxide production from air: Using pulsed powered gliding arc reactor for a containerized plant
Publication TypeJournal Article
Year of Publication2018
AuthorsB.S Patil, F.JJ Peeters, G.J van Rooij, J.A Medrano, F. Gallucci, J. Lang, Q. Wang, V. Hessel
JournalAIChE Journal
Volume64
Issue2
Pagination526-537
Keywordscontainerized process plant, high speed imaging, milliscale gliding arc reactor, nitrogen fixation, pulsed powered
Abstract

The production of NOx from air and air + O2 is investigated in a pulsed powered milli-scale gliding arc (GA) reactor, aiming at a containerized process for fertilizer production. Influence of feed mixture, flow rate, temperature, and Ar and O2 content are investigated at varying specific energy input. The findings are correlated with high-speed imaging of the GA dynamics. An O2 content of 40–48% was optimum, with an enhancement of 11% in NOx production. Addition of Ar and preheating of the feed resulted in lower NOx production. Lower flow rates produced higher NOx concentrations due to longer residence time in the GA. The volume covered by GA depends strongly on the gas flow rate, emphasizing that the gas flow rate has a major impact on the GA dynamics and the reaction kinetics. For 0.5 L/min, 1.4 vol % of NOx concentration was realized, which is promising for a containerized process plant to produce fertilizer in remote locations. © 2017 American Institute of Chemical Engineers AIChE J

DOI10.1002/aic.15922
Division

MaSF

Department

NFC

PID

f894301e083323f4019f60100d1c725d

Alternate TitleAIChE J.

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